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The electrophilic activation of the two C=O double bonds of CO2 in the cycloaddition reactions involved in the domino reaction between methyl isocyanide, acetylenedicarboxylate and CO2 yielding a spiro-compound has been studied within the Molecular Electron Density Theory (MEDT) at the MPWB1K/6-311G(d,p) computational level. The approaching mode of the carbonyl groups of CO2 and lactone to the high...
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