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The mechanistic dichotomy between concerted E2 and stepwise E1cb of the base‐promoted elimination of 2‐aryl‐3‐chloro‐2‐R‐propanols was examined computationally at the HF, M05‐2X, and MP2 levels of theory. Optimizations of transition states (TSs) and reaction intermediates, and intrinsic reaction coordinates (IRC) calculations showed that there was a single reaction route for each substrate, and that...
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