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Anchoring a layer of amorphous hydrogel on an antagonistic elastomer holds potential applications in surface aqueous lubrication. However, the interfacial crack propagation usually occurs under continuous loads for amorphous hydrogel, leading to the failure of hydrogel interface. This work presents a universal strategy to passivate the interfacial cracks by designing a hydrogen bonds‐pinned entanglement...
A seamless and tough interface to integrate incompatible/immiscible soft materials is highly desired for flexible/wearable electronics and many soft devices with multi‐layer structures. Here, a surfactant‐mediated interfacial chemistry is introduced to achieve seamless and tough interfaces in soft multi‐layer structures, with an ultra‐high interfacial toughness up to ≈1300 J m−2 for the architectural...
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