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An amazing phenomenon of the relative magnitude of modulus of two liquid‐crystal (LC) gels is found inverted under/above their phase transition temperature TLC‐iso, which is further proved to be caused by their diverse morphology flexibility. By testing the polarity of two LCs, gelator POSS‐G1‐Boc (POSS=polyhedral oligomeric silsesquioxane) was discovered to self‐assemble into more flexible structures...
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