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Using the time‐dependent quantum wave packet method, the photoassociation (PA) processes of He + H
+→ HeH+ and He + D
+→ HeD+, driven by the sin2‐shaped femtosecond laser pulse in the electronic ground state, including multiphoton transitions and dissociations, are investigated for a wide range of initial collision momenta spanning from 1 to 4 a.u. (or for the collision energy roughly in the ranges...
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