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Multiphase coexistence is the key to rendering samples with superior piezoelectric properties for BaTiO3 ceramics. Ba(Ti1−xSnx)O3 (BTS, x = 0.0–0.30) ceramics are prepared by the traditional solid‐state method. Orthorhombic (O) and tetragonal (T) phases are visually observed to coexist only in the ceramics with the low‐doping of Sn (x = 0.025–0.075) by electron backscattered diffraction (EBSD). The...