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The relationship among the sintering behavior, crystal structure, chemical bonding properties, and dielectric properties of wolframite‐type ZnZr(Nb1−xTax)2O8 (0.0 ≤ x ≤ 1.0) ceramics was investigated with the progressive replacement of Nb5+ by Ta5+. The optimum sintering temperature increases from 1225 to 1375°C with increasing Ta5+ content. The εr value falls from 27.34 to 22.34 due to a gradual...
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