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Utilizing both cationic and anionic oxygen redox reactions is regarded as an important approach to exploit high‐capacity layered cathode materials with earth abundant elements. It has been popular strategies to effectively elevate the oxygen redox activities by Li‐doping to introduce unhybridized O 2p orbitals in NaxMnO2‐based chemistries or enabling high covalency transition metals in P2‐Na0.66Mn...
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