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A method to produce highly efficient and long‐range vertical charge transport is demonstrated in an undoped polythiophene thin film, with average mobilities above 3.1 cm2 V−1 s−1. These record high mobilities are achieved by controlled orientation of the polymer crystallites enabling the most efficient and fastest charge transport along the chain backbones and across multiple chains. The significant...
Vertical chain backbone alignment in a semiconducting polythiophene film is illustrated by D. R. Barbero and co‐workers on page 2359. The chain alignment enables fast charge transport and ultrahigh mobility, reaching a record high average mobility of 3.1 cm2 V−1 s−1 in the vertical direction, showing that mobilities comparable to those of inorganic materials can be obtained over relatively large distances...
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