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In article number 1905825, Yuan Qiu, Xijun Liu, and co‐workers design a simple yet novel strategy to develop oxygen‐doped Nb4N5 by introducing nitrogen‐vacancy. The catalyst exhibits efficient performance for selective conversion of CO2 to CO and simultaneous excellent durability. The work provides a new perspective for an in‐depth understanding toward the structure–activity relationship between defects...
Surface vacancy engineering holds great promise for boosting the electrocatalytic activity for CO2 reduction reaction; however, the vacancies are generally unstable and may degrade into the inactive phase during electrolysis. Stabilizing the vacancy‐enriched structure by heteroatoms can be an effective strategy to get a robust and active catalyst. Herein, a nitrogen‐vacancy enriched Nb4N5 on N‐doped...
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