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Ferro‐pyro‐phototronic (FPP) effect is a triple coupling of ferroelectricity, light‐induced pyroelectricity, and photo‐excitation, which holds a bright promise for next‐generation modern optoelectronic devices. However, except for few oxides (e.g., BaTiO3), new FPP‐active candidates remain extremely scarce due to the knowledge lacking on the underlying role of three coupling components. By tailoring...
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