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Semiclathrate-based CO2 capture from flue gas in the presence of various quaternary ammonium salts (QASs) such as tetra-n-butyl ammonium bromide (TBAB), tetra-n-butyl ammonium chloride (TBAC), and tetra-n-butyl ammonium fluoride (TBAF) was investigated with a primary focus on the thermodynamic, kinetic, and spectroscopic aspects. The thermodynamic stability of the CO2 (20%)+N2 (80%)+QAS semiclathrates...
The enclathration of guest gases such as CH4 and CO2 in tetra-n-butyl ammonium chloride (TBAC) semiclathrates and their potential application to natural gas storage and CO2 capture were examined with a primary focus on stability condition measurements and cage filling characteristics. The phase behaviors clearly demonstrated that the double CH4 (or CO2)+TBAC semiclathrates yielded a significantly...
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