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In article number 2003945, Qi Zhang, Shaoming Huang, and co‐workers develop a molecular‐level interface engineering strategy with long‐chain Lewis bases to optimize long‐distance ion transport across interfaces in solid electrolytes consisting of metal‐organic frameworks. The engineered solid electrolyte demonstrates single ion transport capability and higher ion conductivity and endows the solid‐state...
Metal–organic frameworks (MOFs) have drawn considerable interest as solid electrolytes (SEs) by virtue of their talents for rational design as ion channels. The crystal interface plays a significant role in ion transport and is thus of vital importance to the performance of solid batteries, however, interface effects of MOFs in SEs are not yet fully understood, especially at the molecular level, and...
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