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The realization of efficient large‐area perovskite solar cells stands as a pivotal milestone for propelling their future commercial viability. However, the upscaling fabrication of perovskite solar cells is hampered by efficiency losses, and the underlying growth mechanism remains enigmatic. Here, it is unveiled that a prevalent upscaling technology, namely blade‐coating, inherently triggers top‐down...
Ruddlesden–Popper (RP) faults are well known in oxide perovskites, and are also observed in promising metal halide perovskites. However, the effect of RP faults on optical properties of perovskite has not been systematically investigated. In this study, it is found that RP faults are common planar faults in all‐vacuum deposited CsPbBr3‐based perovskite polycrystal thin films, and the density of RP...
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