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The significance of second‐sphere interactions in synthetic catalysts and metalloenzyme active sites has encouraged the development of ligand frameworks capable of supporting intramolecular hydrogen‐bonding networks. With this approach in mind, we prepared a series of 2,6‐pyridinedicarboxamide ligands (H2LX) that feature outer‐sphere heterocyclic groups (pyridine, pyrimidine, or quinoline rings)....
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