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Replacing oxygen with sulfur in a squaraine bridge compound leads to a large increase in triplet yield (and triplet-state absorption) while maintaining the already enhanced two-photon absorption as well as the singlet excited-state absorption.
We compare GaAs and GaN for IR detection using extremely non-degenerate two-photon absorption. While the small gap material has larger ND-2PA and hence better sensitivity to IR, unwanted background from degenerate 2PA outweighs this advantage.
Using extremely nondegenerate photons in frequency (energy ratios >10/1), we measure 2–4 orders of magnitude enhancement of two-photon absorption in semiconductors compared to the degenerate case. We demonstrate sub-femtosecond gated detection directly on semiconductor diodes.
We report the two-photon absorption spectrum of single crystals of an asymmetric cyanine-like dye in comparison to its spectrum in solution. The 2PA peak magnitude is comparable to bulk semiconductors of similar absorption edge.
Förster resonance energy transfer from a two-photon absorber to a photochromic spirooxazine are investigated by one- and two-photon absorption. Upon energy transfer, fluorescence of the donor is quenched while that of the photochromic is enhanced.
We performed a detailed experimental investigation and quantum-chemical analysis of a new series of near IR polymethine dyes with 5-butyl-7,8-dihydrobenzo[cd]furo[2,3-f]indolium terminal groups. We also synthesized and studied two neutral dyes, squaraine and tetraone, with the same terminal groups and performed a comparison of the spectroscopic properties of this set of “near IR” dyes (polymethine,...
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