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A major handicap towards the exploitation of radicals is their inherent instability. In the paramagnetic azafullerenyl radical C59N., the unpaired electron is strongly localized next to the nitrogen atom, which induces dimerization to diamagnetic bis(azafullerene), (C59N)2. Conventional stabilization by introducing steric hindrance around the radical is inapplicable here because of the concave fullerene...
Ein Komplex aus [10]Cycloparaphenylen ([10]CPP) mit dem Bisazafulleren (C59N)2 wurde experimentell und computerchemisch untersucht. In dieser Struktur sind zwei [10]CPP‐Ringe an das dimere Azafulleren gebunden, [10]CPP⊃(C59N)2⊂[10]CPP. Die beobachteten photophysikalischen und Redox‐Eigenschaften lassen auf eine elektronische Interaktion zwischen den Komponenten schließen, insbesondere mit dem zweiten...
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