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Fine tuning of cascade reaction pathways: The allene core of 1,3‐di‐tert‐butyl‐1,3‐diethynylallenes has been shown in the past to be essentially unreactive. However, its inherent reactivity could be unleashed by the introduction of tailored substituents to induce a variety of highly selective reaction cascades (e.g. 4π electrocyclization, see scheme). These novel processes provide rapid access to...
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