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A polyhedral oligomeric silsesquioxane-[60]fullerene (POSS-C60) dyad was designed and used as a novel electron acceptor for bulk heterojunction (BHJ) polymer solar cells (PSCs) with an inverted device configuration. The studies of time-resolved photoinduced absorption of the pristine thin film of poly[(4,4′-bis(2-ethylhexyl)dithieno[3,2-b:2′,3′-d]silole)-2,6-diyl-alt-(4,7-bis (2-thienyl)-2,1,3-benzothiadiazole)-5,5′-diyl]...
With a supramolecular “double‐cable” structure in the solid state, a light harvesting porphyrin‐fullerene dyad is demonstrated to be a promising candidate for new electron acceptors in high‐performance bulk heterojunction (BHJ) polymer solar cells (PSCs). It has long‐lived mobile carriers, a high short circuit current, and a large open circuit voltage.
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