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Two new amino core‐substituted naphthalene diimides (cNDIs) bearing fluorinated side chains have been synthesised. Steady‐state and time‐resolved fluorescence spectroscopy reveals unprecedented optical properties for the cNDIs with high quantum yields of ∼0.8 and fluorescence lifetimes of ∼13 ns in a range of solvents. These properties are apparent at the level of single molecules, where the compounds...
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