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High‐valent metal–oxygen species (M–O–X species, as opposed to terminal metal‐oxo, M=O, species) have been found to constitute a large family of capable oxidants. Herein, synthetic high‐valent complexes with hydroxide, alkoxide and other anionic O‐atom ligands, as well as O–Lewis acid adducts, are reviewed with a focus on their reactivity. Mn, Fe and Ru complexes are described, as well as recent additions...
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