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Thermal rearrangement of substituted N-acyl-2,2-dimethyl aziridines: a mechanistic study. The thermolysis of N-acyl-2,2-dimethyl aziridines 1 yielded N-methallyl amides 2 and/or oxazolines 3 depending on their substitution. These results suggest the intermediate formation of a zwitterion 1′ by heterolytic cleavage of the CMe 2 –N bond of aziridines 1, which could evolve either through hydrogen...
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