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Reduction of the bis‐(pyrazolyl)pyridine complex [LCr]2 with stoichiometric KC8 in THF produces a species that is reactive with CO2 to produce an aggregate composed of paramagnetic K2L2Cr2(CO3) linked by KCl into a product of formula [K2L2Cr2(CO3)]4⋅2KCl. X‐ray diffraction reveals a pincer hydrocarbon exterior and an inorganic interior composed of K+, Cl− and carbonate oxygens. Every Cr is five coordinate...
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