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A nonmagnetic compound, [NO 2 BzPy][Cu(mnt) 2 ] (mnt 2− =maleonitriledithiolate; NO 2 BzPy + =1-(4′-nitrobenzyl)pyridinium), is isostructural with [NO 2 BzPy][Ni(mnt) 2 ], which is a quasi-1D spin system and exhibits a spin-Peierls-like transition with J=192K in the gapless state and spin energy gap=738K in the dimerization state, respectively...
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