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Investigations on the factors that govern unusual branched alkylation of 2‐aroylbenzofurans with acrylates by Ru‐catalyzed carbonyl‐directed C−H activation has been carried out by calculating the kinetics associated with the two key steps—the coordination of the acrylate with the intermediate ruthenacycle and the subsequent migratory insertion reaction—studied with the help of DFT calculations. Eight...
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