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Systemchemie T.‐Y. D. Tang et al. berichten in der Zuschrift auf S. 6006, dass sich die pH‐Responsivität eines Polykations nutzen lässt, um eine Flüssig‐flüssig‐ Phasentrennung unter Bildung von Koazervattröpfchen innerhalb von Lipidvesikeln zur Steuerung der Enzymaktivität anzutreiben.
In situ, reversible coacervate formation within lipid vesicles represents a key step in the development of responsive synthetic cellular models. Herein, we exploit the pH responsiveness of a polycation above and below its pKa, to drive liquid–liquid phase separation, to form single coacervate droplets within lipid vesicles. The process is completely reversible as coacervate droplets can be disassembled...
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