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Recent wide-band (65–850 GHz) electron magnetic resonance (EMR) study determined the zero field splitting (ZFS) parameters (ZFSPs) for Fe2+ in natural and synthetic forsterite (Mg2SiO4) based on the fictitious spin S′ = 1 approach. So-obtained ZFSPs (D′, E′) are incompatible with those available in literature for 3d6 (Fe2+) and 3d4 (Fe4+, Mn3+, Cr2+) ions with the electronic spin S = 2, which predominantly...
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