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Nematic liquid crystals (NLCs), 4‐cyano‐4′‐pentylbiphenyl and 4‐cyano‐4′‐octylbiphenyl, were applied as additives to polymer solar cells with P3HT:PC61BM blend films. The incorporation of NLC additives led to a higher absorbance of the blend film, a higher crystallinity of P3HT, closer P3HT chains, larger PC61BM domains and enhanced hole/electron mobilities even without post‐thermal annealing. The...
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