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The subcomponent self‐assembly of a bent dialdehyde ligand and different cationic and anionic templates led to the formation of two new metallosupramolecular architectures: a FeII4L6 molecular rectangle was isolated following reaction of the ligand with iron(II) tetrafluoroborate, and a M5L6 trigonal bipyramidal structure was constructed from either zinc(II) tetrafluoroborate or cadmium(II) trifluoromethanesulfonate...
The reaction of 2,6‐diformylpyridine with diverse amines and PdII ions gave rise to a variety of metallosupramolecular species, in which the PdII ion is observed to template a tridentate bis(imino)pyridine ligand. These species included a mononuclear complex as well as [2+2] and [3+3] macrocycles. The addition of pyridine‐containing macrocyclic capping ligands allows for topological complexity to...
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