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Developing new asymmetric auto‐tandem catalysis processes, especially in a divergent manner, is highly attractive but extremely challenging. Presented herein is a palladium‐catalyzed auto‐tandem reaction between 2,4‐dienyl carbonates and o‐TsNH arylimines or trifluoroacetophenones that proceeds through a consecutive N‐allylation, vinylogous addition, π‐σ‐π isomerization, and another N‐allylation sequence...
Developing new asymmetric auto‐tandem catalysis processes, especially in a divergent manner, is highly attractive but extremely challenging. Presented herein is a palladium‐catalyzed auto‐tandem reaction between 2,4‐dienyl carbonates and o‐TsNH arylimines or trifluoroacetophenones that proceeds through a consecutive N‐allylation, vinylogous addition, π‐σ‐π isomerization, and another N‐allylation sequence...
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