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The CO2 electroreduction to fuels is a feasible approach to provide renewable energy sources. Therefore, it is necessary to conduct experimental and theoretical investigations on various catalyst design strategies, such as electronic metal–support interaction, to improve the catalytic selectivity. Here a solvent‐free synthesis method is reported to prepare a copper (Cu)‐based metal–organic framework...
The CH activation in the tandem, “merry‐go‐round”, [(dppp)Rh]‐catalyzed (dppp=1,3‐bis(diphenylphosphino)propane), four‐fold addition of norborene to PhB(OH)2 has been postulated to occur by a C(alkyl)H oxidative addition to square‐pyramidal RhIIIH species, which in turn undergoes a C(aryl)H reductive elimination. Our DFT calculations confirm the RhI/RhIII mechanism. At the IEFPCM(toluene, 373...
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