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Metal‐mediated base pairs have been extensively utilized in many research fields, including genetic‐code extension, novel therapeutics development, and nanodevice design. Compared to other cations, AgI is more flexible in pairing with natural base pairs. Herein, we present a DNA structure containing two C‐AgI‐C pairs and the first reported G‐AgI‐G pair in a short 8mer DNA strand. This structure not...
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