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A non‐aromatic expanded carbaporphyrinoid, incorporating two built‐in 2,7‐pyrenylene moieties was synthesized. The intrinsically labile structure was demonstrated by proton‐triggered conformational changes between the figure‐of‐eight and quasi‐Möbius conformers. Upon treatment with Pd(OAc)2, the reaction produces two bis‐PdII complexes with distinct coordination modes. Metal coordination serves to...