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A large nonlinear optical (NLO) coefficient and a wide band gap are two crucial but contradictory parameters that are difficult to achieve simultaneously in a single infrared (IR) NLO compound. A salt‐inclusion chalcogenide (SIC), Li[LiCs2Cl][Ga3S6] (1), was prepared that presents a nanosized tunnel framework constructed from monotype chalcogenide tetrahedra. Highly oriented covalent GaS4 tetrahedra...
Ein neues Chalkogenid mit Salzeinschluss, beispiellosem 3D‐[Ga3S6]‐Gerüst und nm‐großen Tunneln wird von X.‐M. Jiang, G.‐C. Guo et al. in ihrer Zuschrift auf S. 4886 vorgestellt. Der kovalente Wirt und die ionischen Gäste tragen synergistisch zur großen nichtlinear‐optischen (NLO), effizienten und ultraweiten Bandlücke bei. Dies ist vielversprechend für Anwendungen in IR‐NLO‐Materialien.
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