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Perovskites are attracting attention for optoelectronic devices. Despite their promise, the large‐scale synthesis of perovskite materials with exact stoichiometry, especially high‐entropy perovskites, has been a major challenge. Moreover, the difficulty in stoichiometry control also hinders the development of perovskite X‐ray flat‐panel detectors. Previous reports all employed simple MAPbI3 as the...
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