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Ionizable cationic lipids are recognized as an essential component of lipid nanoparticles (LNPs) for messenger RNA (mRNA) delivery but can be confounded by low lipoplex stability with mRNA during storage and in vivo delivery. Herein, the rational design and combinatorial synthesis of esterase‐triggered decationizable quaternium lipid‐like molecules (lipidoids) are reported to develop new LNPs with...
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