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Porous heterostructured electrocatalysts with multifunctionality and synergistic effect have much benefit for efficient electrocatalytic CO2 reduction reaction (CO2RR), yet it still remains a daunting challenge to explore heterostructures based on covalent organic frameworks (COFs) and metal–organic frameworks (MOFs) in this field. Here, a series of honeycomb‐like porous crystalline hetero‐electrocatalysts...
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