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Ultrastrong bioinspired graphene‐based fibers are designed and prepared via synergistic toughening of ionic and covalent bonding. The tensile strength reaches up to 842.6 MPa and is superior to all other reported graphene‐based fibers. In addition, its electrical conductivity is as high as 292.4 S cm−1. This bioinspired synergistic toughening strategy supplies new insight toward the construction of...
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