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The NO–CO reaction kinetics has been studied on Pd/MgO (100) model catalysts at low pressure by a pulsed molecular beam technique. The model catalysts have been prepared by epitaxial growth of metal clusters in UHV on cleaved MgO single crystals. Three samples with mean clusters sizes of 2.8, 6.9 and 15.6nm have been studied. The reaction products are mainly N 2 and CO 2 . The steady-state...
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