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Perovskite single‐crystal redissolution (PSCR) strategy is highly desired for efficient formamidinium lead triiodide (FAPbI3) perovskite photovoltaics with enhanced phase purity, improved film quality, low trap‐state density, and good stability. However, the phase transition and crystallization dynamics of FAPbI3 remain unclear in the PSCR process compared to the conventional fabrication from the...
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