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Monomer design strategy has become a powerful tool to access polymers with desired and diverse functionalities. Here, we designed a novel monomer 2‐((benzyloxy)methyl)‐1,4‐oxathiepan‐7‐one (BTO) via installing a benzyl ether side chain to the structure of 1,4‐oxathiepan‐7‐one (OTO). The ring‐opening polymerization of BTO with Zn1 as the catalyst demonstrated the characteristics of living polymerization...
A synthetic strategy for catalytic asymmetric conjugate addition‐protonation and diastereoselective switch between 5H‐oxazol‐4‐ones and 5‐methylene 1,3‐oxazolidine‐2,4‐diones was established. An array of chiral conjugate addition‐protonation products bearing 1,3‐O‐heterotertiary‐O‐heteroquarternary nonadjacent stereocenters were obtained in excellent yields, moderate to good diastereoselectivities,...
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