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We report experimental and theoretical investigations of monolayer MoO 3 nanocrystals grown on Au(111), in contrast to the bilayered structure of the bulk oxide crystal. The Au surface acts as the other half of the bilayer by satisfying local bonding requirements through charge redistribution at the interface. Epitaxy with the Au lattice is achieved through the ability of the Mo–O bonds to...
We have developed a synthetic procedure that yields novel nanocrystalline, islands of MoO3 on Au(111). Careful control of the growth conditions yields monolayer islands with a rectangular unit cell that is aligned with the Au substrate. These structures are distinctly different than either bulk MoO3 or than ramified, two-dimensional MoO3 islands formed on Au(111) which were recently reported [J. Am...
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