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The TFA‐prompted/Rh(III)‐catalysed chemoselective C3−H alkylation, C2−H dienylation and cyclopropylation of indoles have been realized by virtue of methylenecyclopropanes as the versatile coupling partners. This protocol features broad substrate/functional group compatibility and tunable regio‐/chemoselectivity. Diversified derivatization of the obtained products has been also successfully demonstrated,...