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1,3‐Allyl and 1,2‐allyl shifts through [3,3]‐ and [2,3]‐sigmatropic rearrangements are well‐established and widely used in organic synthesis. In contrast, 1,5‐allyl shift through related [3,5]‐sigmatropic rearrangement is unknown because [3,5]‐sigmatropic rearrangement is thermally Woodward–Hoffmann forbidden. Herein, we report an unexpected discovery of a formal 1,5‐allyl shift of allyl furfuryl...
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