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Factors affecting the FeIFeI/FeIFe0 reduction potentials (E0) in a series of propane and azadithiolate bridged (µ‐SRS)[Fe(CO)3]2 synthetic model complexes of diiron hydrogenases are investigated. The E0 is found to vary from 60 to 390 mV depending on the nature of the substituent (Alkyl or Aryl) on the nitrogen atom at the bridgehead of the azadithiolate. The E0 is found to shift to more negative...
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