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Single atom sites (SAS) of FeN4 are clarified as one of the most active components for the oxygen reduction reaction (ORR). Effective strategies by engineering the local coordination environment and site density of FeN4 sites are crucial to further enhance the electrocatalytic ORR performance. Herein, the integration of a second metal of Mn with Fe to construct Fe&Mn/N‐C catalysts with enhanced...
The capability of manipulating the interfacial electronic coupling is the key to achieving on‐demand functionalities of catalysts. Herein, it is demonstrated that the electronic coupling of Fe2N can be effectively regulated for hydrogen evolution reaction (HER) catalysis by vacancy‐mediated orbital steering. Ex situ refined structural analysis reveals that the electronic and coordination states of...
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