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The synthesis of a novel 1-acyl-thiourea species (C 14 H 17 N 2 O 2 SCl), has been tailored in such a way that two distinct NH⋯OC intramolecular competing hydrogen bonds are feasible. The X-ray structure analysis as well as the vibrational (FT-IR and FT-Raman) data reveal that the S conformation is preferred, with the CO and CS bonds of the acyl-thiourea group pointing...
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