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A facile strategy is developed to fabricate a two‐layer grafted polymer coatings on silicon wafers, specifically soft crosslinked polythioether as middle damping layer and stiff poly(methyl methacrylate) (PMMA) as top protecting layer. At first, a highly crosslinked polythioether layer was constructed on the surface of the silicon wafer with tunable thickness and smooth morphology with trimethylolpropane...