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Den Zufall ausgefroren: Durch topotaktische Hydridreduktion gelang die Synthese der vollständig reduzierten Stammphase Sr4Fe6O12 der wichtigen Verbindungsfamilie Sr4Fe6O13±δ. Als eine von wenigen zeigt die Struktur Paare kantenverknüpfter Tetraeder, die in diesem Fall bei 300 K zufällig verteilte FeII‐ und FeIII‐Zentren enthalten. Beim Abkühlen kommt es zu einer Ladungsordnung, sodass jedes Tetraederpaar...
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