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An intriguing structural transition from the quasi‐planar form of B12 cluster upon the interaction with lithium atoms is reported. High‐level computations show that the lowest energy structures of LiB12, Li2B12, and Li3B12 have quasi‐planar (Cs), tubular (D6d), and cage‐like (Cs) geometries, respectively. The energetic cost of distorting the B12 quasi‐planar fragment is overcompensated by an enhanced...
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